Mr Annan cautioned both nations that the issue could propagate across the area if the assault was not ceased.
The trip came after shares with Syrian Chief executive Bashar al-Assad on Thursday which he described as "constructive".
Meanwhile, Italy is submitting warships to its naval platform at Syria's slot of Tartus, army resources said.
Correspondents say the shift is developed to demonstrate that Italy - an best friend of the Syrian govt - will secure its passions in the area.
'New approach'
After conference International Reverend Ali Akbar Salehi in Tehran on Wed, Mr Annan said he was looking for Iran's "support and co-operation" to take care of the disaster.
He said Tehran could perform a "positive role" in assisting end the bloodshed.
Mr Salehi informed correspondents that his nation was "part of the solution".But the US, which accuses Iran of offering support to Damascus, throw down on the declare.
Activists said assault on Thursday stated many more lives
"I don't think anybody with a immediately experience could dispute that Iran has had a good effect on improvements in Syria," White-colored Home spokesperson Jay Carney said on Wed.
Later, Mr Annan moved down in Baghdad for a conference with Iraqi Excellent Reverend Nouri Maliki.
The former UN assistant common said the two men had mentioned "the need to do everything possible to quit the killing", but did not intricate.
Mr Annan is predicted to brief the UN Protection Authorities in New You are able to on the result of this newest circular of shares from his Geneva platform on Wed.
He has confessed his strategy to discover a governmental remedy in Syria has not won. A ceasefire was predicted to start in mid-April as aspect of his six-point serenity effort.
Following shares with Chief executive Assad on Thursday, Mr Annan said the couple had decided a new strategy to finishing the assault.
"We decided an strategy which I will discuss with the equipped resistance," he said in Damascus.
"I also burdened the value of going forward with a governmental conversation, which obama allows."
President Assad had recommended finishing the issue "step by step", Mr Annan said.
This would include trying to contain the assault in the toughest impacted places and developing on it "from the earth up".
But even with few information, many experts have indicated issue that any such strategy would be successful.
Meanwhile, the issue stated more life on Wed, along with a participant of the Syrian Arabic Red Cres.
'Significant deployment'
President Assad said on Weekend he still had the support of the Syrian people
The assault also once again built into Lebanon, with capturing and placing by Syrian causes being revealed in south places. Lebanon said it would deliver more soldiers to strengthen the boundary.
Meanwhile, Italy has sent a naval flotilla of seven warships led by an anti-submarine destroyer to its Syrian platform at Tartus, according to Interfax information organization.
The US said it was conscious of the shift, but did not see cause for issue.
According to resources mentioned by Interfax, the delivers were holding maritime on a exercising objective, as well as meals and petrol for the servicing and fix platform.
BBC diplomatic reporter Jonathan Marcus says that, by any requirements, the flotilla is a considerable naval implementation.
He says Moscow seems to be submitting a indication to the Syrian program that it is placing a power into the Med sea that could be used to extricate European employees and devices from their naval platform, should it be needed.
Equally Moscow is signalling to the US and the Western that it plans to secure its passions in the area, our reporter contributes.
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